MgO support mediated enhancement of La2BMnO6 (B = Co, Ni) perovskite oxide in catalytic combustion of propane
الموضوعات : Iranian Journal of CatalysisHamidreza Roozbahani 1 , Sarah Maghsoodi 2 , Behrouz Raei 3 , Amirhossein Shahbazi Kootenaei 4 , Zoha Azizi 5
1 - Department of Chemical Engineering, Mahshahr Branch, Islamic Azad University, Mahshahr, Iran.
2 - Department of Chemical Engineering, Mahshahr Branch, Islamic Azad University, Mahshahr, Iran.
3 - Department of Chemical Engineering, Mahshahr Branch, Islamic Azad University, Mahshahr, Iran.
4 - Department of Chemical Engineering, Mahshahr Branch, Islamic Azad University, Mahshahr, Iran.
5 - Department of Chemical Engineering, Mahshahr Branch, Islamic Azad University, Mahshahr, Iran.
الکلمات المفتاحية: propane, Support, catalytic combustion, Double perovskite oxide, Composite oxide,
ملخص المقالة :
Perovskite oxides possessing high stability and composition adjustability are effective in many applications. The La2BMnO6 (B=Co, Ni) double perovskite oxides were synthesized using the sol-gel method and deposited on MgO support (loading = 10, 20, and 30 wt. %) using a mechanical mixing method by an ultrasonic device. The elaborated samples were investigated for application in propane deep oxidation. The catalytic performance of these catalysts was analyzed by a variety of characterization techniques such as XRD, SEM, FTIR, TEM, and H2-TPR. Ni-containing catalysts were found to have superior catalytic activity than the sample containing Co. The lowest catalytic activity belonged to the cobalt-containing double perovskite with 10 wt.% loading on MgO support, while the highest conversion was related to the 20La2NiMnO6/MgO composite oxide with T90 = 434 °C. The support showed a positive impact on the performance of the catalysts. Deposition of a certain amount of perovskite oxides on the support boosted the specific surface area of the catalyst and, therefore, combined with improved reducibility, improved propane catalytic degradation.
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