• الصفحة الرئيسية
  • جذب فلز منگنز(II) و حذف رنگزای Reactive Black B با تلفیق فرایندهای جذب بیولوژیکی و UV/H2O2 در راکتور واحد از پساب

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رقم المقالة : JEST-1702-3381 (R1) زيارة : 143 الصفحة: 29 - 42

10.22034/jest.2020.24750.3381

نوع المخطوط: ابحاث

جذب فلز منگنز(II) و حذف رنگزای Reactive Black B با تلفیق فرایندهای جذب بیولوژیکی و UV/H2O2 در راکتور واحد از پساب

الموضوعات :

رعنا خلیل نژاد 1 , رضا مرندی 2 , مرتضی خسروی 3

1 - دکترای تخصصی شیمی کاربردی، مدرس مدعو، دانشگاه پیام نور، تهران، ایران*(مسوول مکاتبات).
2 - دکترای تخصصی مهندسی محیط زیست، دانشیار، عضو هیات علمی دانشگاه آزاد واحد تهران شمال.
3 - دکترای تخصصی شیمی پلیمر، استاد، عضو هیات علمی دانشگاه آزاد واحد تهران شمال.

تاريخ الإرسال : 13 الجمعة , جمادى الأولى, 1438 تاريخ التأكيد : 24 الأربعاء , ذو القعدة, 1438 تاريخ الإصدار : 25 الجمعة , ربيع الأول, 1441

الکلمات المفتاحية: جذب بیولوژیکی, راکتور, سدیم آلژینات, تلفیقی, فرایند,

ملخص المقالة :

زمینه و هدف: فلزات سنگین و رنگزاها به وسیله فعالیت های صنعتی و توسعه فن آوری بیشتر از میزان طبیعی در محیط زیست منتشر شده اند. این آلاینده ها به دلیل سمی بودن، اثرات نابهنجاری بر محیط زیست و سلامتی موجودات به ویژه انسان ها دارند. بنابراین توسه روش هایی نوین که بتواند این آلاینده ها را از محیط زیست به طور همزمان حذف کند بسیار مهم است. روش بررسی: در این تحقیق دو روش اکسیداسیون پیشرفته و جذب بیولوژیکی در راکتور واحد تلفیق گردیده و آلاینده ها را وارد راکتور کرده و در صد حذف آن ها بررسی گردید، آلاینده هایی که در این راکتور حذف می شوند رنگزَای Reactive Black B(RBB) و یون منگنز می باشد . برای حذف رنگزای RBB از فرایند UV/H2O2 و برای حذف یون منگنز از جاذب بیولوژیکی که در سدیم آلزینات تثبیت شده بود، استفاده گردید. بعد از انجام دو فرایند مذکور در سیستم batch و با توجه به شرایط بهینه در راکتور واحد این دو فرایند با هم تلفیق شده وگرانول ها را در فیلتر پلی اتیلنی ریخته و در داخل راکتوری که در مرکز آنلامپUVتعبیه شده، قرار گرفت. یافته ها: با توجه به نتایج TOC و COD مشخص گردید که در حالتی که فقط از فرایند UV/H2O2 استفاده شده در صد حذف TOC و COD به ترتیب 35% و 5/79% بوده ولی در حالت تلفیقی درصد کاهش TOC به 56% و COD به 22/90 % می رسد. بحث و نتیجه گیری: به طور همزمان یون منگنز فقط به وسیله گرانول و رنگزا توسط فرایندUV/H2O2و مقدار جزئی توسط گرانول جذب و حذف گردید.

المصادر:


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  12. Hassimi Abu Hasan , H., Sheikh Abdullah, S.R., Tan Kofli,, N., Yeoh, S.J, 2016,  Interaction of environmental factors on simultaneous biosorption of lead and manganese ions by locally isolated Bacillus cereus, Journal of Industrial and Engineering Chemistry 37 , 295–305
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  13. K. Vijayaraghavan, Heng Yun Ni Winnie, R. Balasubramanian,  Biosorption characteristics of crab shell particles for the removal of manganese(II) and zinc(II) from aqueous solutions, Desalination 266 (2011) 195–200
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  15. Marandi. R. 2011. Biosorption of Hexavalent Chromium from Aqueous Solution by Dead Fungal Biomass of Phanerochaete crysosporium: Batch and Fixed Bed Studies.  Chemical Engineering & Technology, Vol. 2, pp.8-22.
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  16. Preetha, B., Viruthagiri, T. 2007, Batch and continuous biosorption of chromium (VI) by Rhizopus Arrhizus, Separation and Purification Technology. Vol. 57, pp. 126–133.
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  17. Ghodbane, H., Hamdaoui, O. 2010. Decolorization of antraquinonic dye, C.I. Acid Blue 25, in aqueous solution by direct UV irradiation, UV/H2O2 and UV/Fe(II) processes, Chemical Engineering Journal, Vol. 160 , pp. 226–231.
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  20. Schrank, S. G., Santos, J. N .R., Santos Souza, D., Santos Souza, E. E. 2007. Decolourisation effects of Vat Green 01 textile dye and textile wastewater using H2O2/UV process, Journal of Photochemistry and Photobiology A: Chemistry. Vol. 186, pp. 125–129
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  21. Huang, Y. H., Tsai, S. T., Huang, Y.F., Chen, C. Y. 2007. Degradation of commercial azo dye reactive Black B in photo/ferrioxalate system, Journal of Hazardous Materials, Vol.140 , pp. 382–388
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  22. Shu, H. Y., Chang, M .C. 2006. Development of a rate expression for predicting decolorization of C.I. AcidBlack 1 in a UV/H2O2 process, Dyes and Pigments, Vol.70, pp. 31-37.
    23.
  23. Yang, Y., Wang, G., Wang, B., Li, Z., Jia, X., Zhou, Q., Zhao, Y., 2011, Biosorption of Acid Black 172 and Congo Red from aqueous solution by nonviable Penicillium YW 01: Kinetic study, equilibrium isotherm and artificial neural network modeling, Bioresource Technology, Vol.102, PP. 828–834. 
    24.
  24. Pathak, C.S., Agarwala, V., Mandal, M.K., 2012, Mechano-chemical synthesis and optical properties of ZnS nanoparticles, Physica B: Condensed Matter., Vol. 407, PP. 3309-3312
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  25. Yang, C., Wang, J., Lei, M., Xie, G., Zeng, G., Luo, S.,2010, Biosorption of zinc(II) from aqueous solution by dried activated sludge, Journal of Environmental Sciences, Vol. 22, PP. 675–680.
    26.
  26. Vijayaraghavan, K., Teo, T. T. 2009. Application of Sargassum biomass to remove heavy metal ions from synthetic multi-metal solution and urban strom water runoff Balasubramanian, R;  Joshi, U.M;  Hazardous Materials, Vol. 164, pp. 1019-1023.
    27.
  27. Joo, J.H., Hassan, S.H.A., Oh, S.E., 2010, Comparative study of biosorption of Zn+2 by Pseudomonas aeruginosa and Bacillus cereus, International Biodeterioration & Biodegradation, Vol. 64, PP. 734-741
    28.
  28. Areco, M.M., Afonso, M.D.S., 2010, Copper, zinc, cadmium and lead biosorption by Gymnogongrus torulosus. Thermodynamics and kinetics studies, Colloids and Surfaces B: Biointerfaces., Vol. 81, PP. 620-628
    29.
  29. Mungasavalli, D. P, Viraraghavan, T,., Jin, Y. C. 2007. Biosorption of chromium from aqueous solutions by pretreated Aspergillus niger: Batch and column studies, Colloids and Surfaces, A: Physicochem. Eng. Aspects, Vol.301, pp. 214–223.
    30.
  30. Han, R., Wang, Y., Yu, W., Zou, W., Shi, J., Liu, H. 2007. Biosorption of methylene blue from aqueous solution by rice husk in a fixed-bed column, Journal of Hazardous Materials, Vol. 141, pp. 713–718.
    31.
  31. Areco, M.M., Afonso, M.D.S. 2010, Copper, zinc, cadmium and lead biosorption by Gymnogongrus torulosus. Thermodynamics and kinetics studies, Colloids and Surfaces B: Biointerfaces, Vol.81, pp. 620-628.
    32.
  32. Zhang, H., Wu, X., Li, X. 2012. Oxidation and coagulation removal of COD from landfill leachate by Fered–Fenton process, Chemical Engineering Journal, Vol. 210, pp.  188-194.
    33.
  33. Xueming Tang, X., Linda, K., Weavers, L.K. 2008. Using photoactivated periodate to decompose TOC from hydrolysates of chemical warfare agents, Journal of Photochemistry and Photobiology A: Chemistry, Vol.194, pp. 212-219.
    34.
  34. Aleboyeh, A., Olya, M.E., Aleboyeh, H. 2008. Electrical energy determination for an azo dye decolorization and mineralization by UV/H2O2 advanced oxidation process, Chemical Engineering Journal, Vol.137, pp. 518–524.
    35.

 

 

_||_

  1. Oller, I., Malato, S., Sanchez-Perez, J.A. 2011. Combination of Advanced Oxidation Processes and biological treatments forwastewater decontamination—A review. Science of the Total Environment. Vol.409, pp.4141-4166.
    2.
  2. Mesdaghinia, A.R., Farrokhi, M., Nasseri, S. 2003. Biodegradability of 2, 4, 6 trichlorophenol (TCP) by fenton, s oxidation process. Hakim Research Journal, Vol. 2(7), pp. 23-40.
    3.
  3. Dixit, A., Tirpude, A. J., Mungray, A.K. 2011. Degradation of 2, 4 DCP by sequential biological–advanced oxidation process usingUASB and UV/TiO2/H2O2, Desalination. Vol. 272, pp. 265-269.
    4.
  4. Lafi, W., Shannak, B., Al-Shannag, M., Al-Anber, Z., Al-Hasan, M. 2009, Treatment of olive mill wastewater by combined advanced oxidation and biodegradation.  Separation and purification Technology, Vol. 70, pp. 141-146.
    5.
  5. Mandal, T., Maity, S., Dasgupta, D., Datta, S. 2010.  Advanced oxidation process and biotreatment: Their roles in combined industrial wastewater treatment. Desalination, Vol. 250, pp. 87-94.
    6.
  6. Moussavi, G., Yazdanbakhsh, A., Heidarizad, M. 2009, the removal of formaldehyde from concentrated synthetic wastewater using O3/MgO/H2O2 process integrated with the biological treatment. Hazardous Materials, Vol. 171, pp. 907-913.
    7.
  7. Barreto-Rodrigues, M., Souza, V. B. J., Silva, E. S., Silva, F. T., Paiva, T. C. B. 2007. Combined photocatalytic and fungal processes for the treatment of nitrocellulose industry wastewater.  Hazardous Materials, Vol. 161, pp. 1560-1573.
    8.
  8. Moradi Pasand, L., Ayati B. 1392. Study of reactive blue 171 dye degradation in hybrid system of UV/H2O2& SBAR. Iran. J. Health & Environ., 2013, Vol.6, No. 3, pp.393-406. (Persian)
    9.
  9. Yao-Hui Huang∗, Shu-Ting Tsai, Yi-Fong Huang, Chuh-Yung Chen. 2007, Degradation of c.ommercial azo dye reactive Black B in photo/ferrioxalate system, Journal of Hazardous Materials, 140, 382–388.
    10.
  10. Sedighi M, khosravi V, Ramedani A, 2012. Estimating the Impact of Important Parameters on Biosorption of Cu and Mn Ions by Bacillus Thuringiensis. NCMBJ. 2 (8) ,45-51. (Persian)
    11.
  11. Fadel, M., Hassanein, N.M., Elshafei, M.M., Mostafa, A.H, Ahmed , M.A.,  Khater, H.M, 2015,  Biosorption of manganese from groundwater by biomass of Saccharomyces cerevisiae Housing and Building National Research Center, 1-8
    12.
  12. Hassimi Abu Hasan , H., Sheikh Abdullah, S.R., Tan Kofli,, N., Yeoh, S.J, 2016,  Interaction of environmental factors on simultaneous biosorption of lead and manganese ions by locally isolated Bacillus cereus, Journal of Industrial and Engineering Chemistry 37 , 295–305
    13.
  13. K. Vijayaraghavan, Heng Yun Ni Winnie, R. Balasubramanian,  Biosorption characteristics of crab shell particles for the removal of manganese(II) and zinc(II) from aqueous solutions, Desalination 266 (2011) 195–200
    14.
  14. Kapoor, A., Viraraghavan, T., Cullimore, D. R. 1999.  Removal of heavy metals the fungus Aspergillus niger.  Bioresource Technology, Vol. 70, pp. 95-104.
    15.
  15. Marandi. R. 2011. Biosorption of Hexavalent Chromium from Aqueous Solution by Dead Fungal Biomass of Phanerochaete crysosporium: Batch and Fixed Bed Studies.  Chemical Engineering & Technology, Vol. 2, pp.8-22.
    16.
  16. Preetha, B., Viruthagiri, T. 2007, Batch and continuous biosorption of chromium (VI) by Rhizopus Arrhizus, Separation and Purification Technology. Vol. 57, pp. 126–133.
    17.
  17. Ghodbane, H., Hamdaoui, O. 2010. Decolorization of antraquinonic dye, C.I. Acid Blue 25, in aqueous solution by direct UV irradiation, UV/H2O2 and UV/Fe(II) processes, Chemical Engineering Journal, Vol. 160 , pp. 226–231.
    18.
  18. Afzal, A., Oppenlander, T. R., Bolton, J., Mohamed Gamal El-Din, M. 2010. Anatoxin-a degradation by Advanced Oxidation Processes: Vacuum-UV at 172 nm, photolysis using medium ressure UV and UV/H2O2. WATER RESERCH, Vol.44 , pp. 278 – 286
    19.
  19. 19.Gul, S. S., Ozcan-Yildirım, O. 2009, Degradation of Reactive Red 194 and Reactive Yellow 145 azo dyes by O3 and H2O2/UV-C processes, Journal Chemical Engineering, Vol. 155, pp. 684–690.
    20.
  20. Schrank, S. G., Santos, J. N .R., Santos Souza, D., Santos Souza, E. E. 2007. Decolourisation effects of Vat Green 01 textile dye and textile wastewater using H2O2/UV process, Journal of Photochemistry and Photobiology A: Chemistry. Vol. 186, pp. 125–129
    21.
  21. Huang, Y. H., Tsai, S. T., Huang, Y.F., Chen, C. Y. 2007. Degradation of commercial azo dye reactive Black B in photo/ferrioxalate system, Journal of Hazardous Materials, Vol.140 , pp. 382–388
    22.
  22. Shu, H. Y., Chang, M .C. 2006. Development of a rate expression for predicting decolorization of C.I. AcidBlack 1 in a UV/H2O2 process, Dyes and Pigments, Vol.70, pp. 31-37.
    23.
  23. Yang, Y., Wang, G., Wang, B., Li, Z., Jia, X., Zhou, Q., Zhao, Y., 2011, Biosorption of Acid Black 172 and Congo Red from aqueous solution by nonviable Penicillium YW 01: Kinetic study, equilibrium isotherm and artificial neural network modeling, Bioresource Technology, Vol.102, PP. 828–834. 
    24.
  24. Pathak, C.S., Agarwala, V., Mandal, M.K., 2012, Mechano-chemical synthesis and optical properties of ZnS nanoparticles, Physica B: Condensed Matter., Vol. 407, PP. 3309-3312
    25.
  25. Yang, C., Wang, J., Lei, M., Xie, G., Zeng, G., Luo, S.,2010, Biosorption of zinc(II) from aqueous solution by dried activated sludge, Journal of Environmental Sciences, Vol. 22, PP. 675–680.
    26.
  26. Vijayaraghavan, K., Teo, T. T. 2009. Application of Sargassum biomass to remove heavy metal ions from synthetic multi-metal solution and urban strom water runoff Balasubramanian, R;  Joshi, U.M;  Hazardous Materials, Vol. 164, pp. 1019-1023.
    27.
  27. Joo, J.H., Hassan, S.H.A., Oh, S.E., 2010, Comparative study of biosorption of Zn+2 by Pseudomonas aeruginosa and Bacillus cereus, International Biodeterioration & Biodegradation, Vol. 64, PP. 734-741
    28.
  28. Areco, M.M., Afonso, M.D.S., 2010, Copper, zinc, cadmium and lead biosorption by Gymnogongrus torulosus. Thermodynamics and kinetics studies, Colloids and Surfaces B: Biointerfaces., Vol. 81, PP. 620-628
    29.
  29. Mungasavalli, D. P, Viraraghavan, T,., Jin, Y. C. 2007. Biosorption of chromium from aqueous solutions by pretreated Aspergillus niger: Batch and column studies, Colloids and Surfaces, A: Physicochem. Eng. Aspects, Vol.301, pp. 214–223.
    30.
  30. Han, R., Wang, Y., Yu, W., Zou, W., Shi, J., Liu, H. 2007. Biosorption of methylene blue from aqueous solution by rice husk in a fixed-bed column, Journal of Hazardous Materials, Vol. 141, pp. 713–718.
    31.
  31. Areco, M.M., Afonso, M.D.S. 2010, Copper, zinc, cadmium and lead biosorption by Gymnogongrus torulosus. Thermodynamics and kinetics studies, Colloids and Surfaces B: Biointerfaces, Vol.81, pp. 620-628.
    32.
  32. Zhang, H., Wu, X., Li, X. 2012. Oxidation and coagulation removal of COD from landfill leachate by Fered–Fenton process, Chemical Engineering Journal, Vol. 210, pp.  188-194.
    33.
  33. Xueming Tang, X., Linda, K., Weavers, L.K. 2008. Using photoactivated periodate to decompose TOC from hydrolysates of chemical warfare agents, Journal of Photochemistry and Photobiology A: Chemistry, Vol.194, pp. 212-219.
    34.
  34. Aleboyeh, A., Olya, M.E., Aleboyeh, H. 2008. Electrical energy determination for an azo dye decolorization and mineralization by UV/H2O2 advanced oxidation process, Chemical Engineering Journal, Vol.137, pp. 518–524.
    35.

 

 

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